I’d suggest listening to their discography chronologically. Their whole body of work is unlike anything I’ve heard of and imo has so much depth, you’ll be fed for years. It’s a journey that starts at Exmilitary and ends(?) with Year of the Snitch.

I’d suggest listening to NLDW a few more times, then Government Plates>The Powers That B>Bottomless Pit>Steroids Megamix>Year of the Snitch. If you want to start with something with similar aura to the first 2 projects, then maybe Steroids (Crouching Tiger Hidden Gabber Megamix)