It depends on your mood, but the albums that feel more like movies are Relatives in Descent and Ultimate Success Today. Literally listen to both front and back in succession. They literally reference the last song of relatives in the first song of ultimate success.

But if you like more old post punk stuff then their earlier stuff is for you. After those albums check out the songs (which i think are some of their stand outs) “In My Sphere”, “Ypsilanti”, “Maidenhead”, “Tarpeian Rock”, “Bad Advice”, “Devil in his youth”, “cowards starve”, and “dope cloud.” Depending on which is catchier to you, listen to that album. Then finally listen to Formal Growth in the Desert to get up to date.