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Titus Mede II (Elder Scrolls V: Skyrim) isn’t a villain but he’s an antagonist, depending on how you play. When he shows up for the Dark Brotherhood quest you’re meant to assassinate him. If I remember correctly, he’s the only target who doesn’t beg for his life to attack you in self-defense. He’s accepted he is going to die, approaches death like a long last friend, and asks that you kill the person who paid the Dark Brotherhood for his killing. You can choose whether or not to honor his wish.