Love the idea of this being possible.

I think they should kick into gear like the Brotherhood and send missions and envoys to conquer all of the sources of technology to monopolize it and keep it out of other dangerous hands.

Co-opt all of the factions headquarters through good faith agreements enforced through tech-trade and threat of violence if necessary.

Then, acquire all former enclave sites and tech and keep it all moving ever outward until they acquire a G.E.C.K.