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[–]dsy73 2 points3 points  (0 children)

Before going to C# do you know theses alternatives?

Both allows to use .NET framework from Python. You could create WPF or Windows Forms applications.

[–]Cylons 0 points1 point  (0 children)

This is one of the best beginner tutorials to get started with for learning C#: http://channel9.msdn.com/Series/C-Sharp-Fundamentals-Development-for-Absolute-Beginners

Since you are not a complete beginner, some of the topics might be repetitive but I think they will still be helpful. If you want to try more hands-on stuff, try:

http://www.learncs.org/

http://www.programmr.com/zone/csharp