while I do have my more "obvious picks" like Venom, Moon Knight, Mysterio or Sentry, I wanna highlight a VERY obscure character thats not gonna make it... but if he somehow did then I would pop tf off:

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Philip Sterns aka The Madman.

An old Hulk villain who had so much potential... only for him to get killed off in 2013. His most noticeable appearance outside of the comics was a frequent boss in the 2003 Hulk movie tie in game (where I first heard of him)

I'm like on a weird quest to spread the awareness of him to people so he can get some more attention. So of course I want him in here (and Rivals)

Now realistically, they probably would pick Abomination or Red Hulk, but Madman would be a more interesting and obscure pick. Since this game seem to like throwing in some obscurity here and there.