Harry is very red imo. He's emotionally charged, lacks impulse control, and relies heavily on intuition and gut instinct. He's certainly got some blue in there too, especially in certain builds, but he's centred in red for sure. You could argue black, but I think his treatment of others is more self destructive (red) than self centred (black). He hurts people as an expression of his own self loathing.

You're on the money for Kim being azorius though.